参考文献

[1]　Boehm H P, Setton R, Stumpp E. Nomenclature and terminology of graphite intercalation compounds（IUPAC Recommendations 1994）[J]. Pure and Applied Chemistry, 1994, 66（9）：1893-1901.

[2]　Novoselov K S, Geim A K, Morozov S V, et al. Electric field effect in atomically thin carbon films[J]. Science, 2004, 306（5696）：666-669.

[3]　Geim A K, Novoselov K S. The rise of graphene[J]. Nature Materials, 2007, 6（3）：183-191.

[4]　Lee C, Wei X D, Kysar J W, et al. Measurement of the elastic properties and intrinsic strength of monolayer graphene[J]. Science, 2008, 321（5887）：385-388.

[5]　Liu F, Ming P B, Li J. Ab initio calculation of ideal strength and phonon instability of graphene under tension[J]. Physical Review B, 2007, 76（6）：064120.

[6]　Lindsay L, Broido D A. Optimized Tersoff and Brenner empirical potential parameters for lattice dynamics and phonon thermal transport in carbon nanotubes and graphene[J]. Physical Review B, 2010, 81（20）：262-265.

[7]　Zandiatashbar A, Lee G H, An S J, et al. Effect of defects on the intrinsic strength and stiffness of graphene[J]. Nature Communications, 2014, 5：3186.

[8]　Min K, Aluru N R. Mechanical properties of graphene under shear deformation[J]. Applied Physics Letters, 2011, 98（1）：013113.

[9]　Zhang Y B, Tan Y W, Stormer H L, et al. Experimental observation of the quantum Hall effect and Berry's phase in graphene[J]. Nature, 2005, 438（7065）：201-204.

[10]　Dawlaty J M, Shivaraman S, Strait J, et al. Measurement of the optical absorption spectra of epitaxial graphene from terahertz to visible[J]. Applied Physics Letters, 2008, 93（13）：131905.

[11]　Nair R R, Blake P, Grigorenko A N, et al. Fine structure constant defines visual transparency of graphene[J]. Science, 2008, 320（5881）：1308.

[12]　Balandin A A, Ghosh S, Bao W Z, et al. Superior thermal conductivity of single-layer graphene[J]. Nano Letters, 2008, 8（3）：902-907.

[13]　Seol J H, Jo I, Moore A L, et al. Two-dimensional phonon transport in supported graphene[J]. Science, 2010, 328（5975）：213-216.

[14]　Ghosh S, Bao W Z, Nika D L, et al. Dimensional crossover of thermal transport in few-layer graphene[J]. Nature Materials, 2010, 9（7）：555-558.

[15]　Ren Y J, Zhu C F, Cai W W, et al. Detection of sulfur dioxide gas with graphene field effect transistor[J]. Applied Physics Letters, 2012, 100（16）：163114.

[16]　Hu S, Lozada-Hidalgo M, Wang F C, et al. Proton transport through one-atom-thick crystals[J]. Nature, 2014, 516（7530）：227-230.

[17]　Zhao W F, Fang M, Wu F R, et al. Preparation of graphene by exfoliation of graphite using wet ball milling[J]. Journal of Materials Chemistry, 2010, 20（28）：5817-5819.

[18]　Su C Y, Lu A Y, Xu Y P, et al. High-quality thin graphene films from fast electrochemical exfoliation[J]. ACS Nano, 2011, 5（3）：2332-2339.

[19]　Chen C H, Yang S W, Chuang M C, et al. Towards the continuous production of high crystallinity graphene via electrochemical exfoliation with molecular in situ encapsulation[J]. Nanoscale, 2015, 7（37）：15362-15373.

[20]　Xia Z Y, Pezzini S, Treossi E, et al. The exfoliation of graphene in liquids by electrochemical, chemical, and sonication-assisted techniques：A nanoscale study[J]. Advanced Functional Materials, 2013, 23（37）：4684-4693.

[21]　Parvez K, Li R J, Puniredd S R, et al. Electrochemically exfoliated graphene as solution-processable, highly conductive electrodes for organic electronics[J]. ACS Nano, 2013, 7（4）：3598-3606.

[22]　Rao K S, Senthilnathan J, Liu Y F, et al. Role of peroxide ions in formation of graphene nanosheets by electrochemical exfoliation of graphite[J]. Scientific Reports, 2014, 4：4237.

[23]　Wang J Z, Manga K K, Bao Q L, et al. High-yield synthesis of few-layer graphene flakes through electrochemical expansion of graphite in propylene carbonate electrolyte[J]. Journal of the American Chemical Society, 2011, 133（23）：8888-8891.

[24]　Yang S, Lohe M R, Müllen K, et al. New-generation graphene from electrochemical approaches：Production and applications[J]. Advanced Materials, 2016, 28（29）：6213-6221.

[25]　Hernandez Y, Nicolosi V, Lotya M, et al. High-yield production of graphene by liquid-phase exfoliation of graphite[J]. Nature Nanotechnology, 2008, 3（9）：563-568.

[26]　Ciesielski A, Samorì P. Graphene via sonication assisted liquid-phase exfoliation[J]. Chemical Society Reviews, 2014, 43（1）：381-398.

[27]　Robinson J A, Wetherington M, Tedesco J L, et al. Correlating Raman spectral signatures with carrier mobility in epitaxial graphene：A guide to achieving high mobility on the wafer scale[J]. Nano Letters, 2009, 9（8）：2873-2876.

[28]　Geim A K. Graphene：Status and prospects[J]. Science, 2009, 324（5934）：1530-1534.

[29]　Yu Q K, Lian J, Siriponglert S, et al. Graphene segregated on Ni surfaces and transferred to insulators[J]. Applied Physics Letters, 2008, 93（11）：113103.

[30]　Zhang Y, Gomez L, Ishikawa F N, et al. Comparison of graphene growth on single-crystalline and polycrystalline Ni by chemical vapor deposition[J]. The Journal of Physical Chemistry Letters, 2010, 1（20）：3101-3107.

[31]　Li X S, Cai W W, An J, et al. Large-area synthesis of high-quality and uniform graphene films on copper foils[J]. Science, 2009, 324（5932）：1312-1314.

[32]　Geng D C, Wu B, Guo Y L, et al. Uniform hexagonal graphene flakes and films grown on liquid copper surface[J]. Proceedings of the National Academy of Sciences of the United States of America, 2012, 109（21）：7992-7996.

[33]　Zeng M Q, Tan L F, Wang J, et al. Liquid metal：An innovative solution to uniform graphene films[J]. Chemistry of Materials, 2014, 26（12）：3637-3643.

[34]　Chen X D, Chen Z L, Jiang W S, et al. Fast growth and broad applications of 25-inch uniform graphene glass[J]. Advanced Materials, 2017, 29（1）：1603428.

[35]　Vlassiouk I V, Stehle Y, Pudasaini P R, et al. Evolutionary selection growth of two-dimensional materials on polycrystalline substrates[J]. Nature Materials, 2018, 17（4）：318-322.

[36]　Cai Z Y, Liu B L, Zou X L, et al. Chemical vapor deposition growth and applications of two-dimensional materials and their heterostructures[J]. Chemical Reviews, 2018, 118（13）：6091-6133.

[37]　He H Y, Klinowski J, Forster M, et al. A new structural model for graphite oxide[J]. Chemical Physics Letters, 1998, 287（1-2）：53-56.

[38]　Paredes J I, Villar-Rodil S, Martínez-Alonso A, et al. Graphene oxide dispersions in organic solvents[J]. Langmuir, 2008, 24（19）：10560-10564.

[39]　Hummers W S Jr, Offeman R E. Preparation of graphitic oxide[J]. Journal of the American Chemical Society, 1958, 80（6）：1339.

[40]　Marcano D C, Kosynkin D V, Berlin J M, et al. Improved synthesis of graphene oxide[J]. ACS Nano, 2010, 4（8）：4806-4814.

[41]　Chen J, Yao B W, Li C, et al. An improved Hummers method for eco-friendly synthesis of graphene oxide[J]. Carbon, 2013, 64：225-229.

[42]　Zhang M, Wang Y L, Huang L, et al. Multifunctional pristine chemically modified graphene films as strong as stainless steel[J]. Advanced Materials, 2015, 27（42）：6708-6713.

[43]　Eigler S, Enzelberger-Heim M, Grimm S, et al. Wet chemical synthesis of graphene[J]. Advanced Materials, 2013, 25（26）：3583-3587.

[44]　Chen J, Zhang Y, Zhang M, et al. Water-enhanced oxidation of graphite to graphene oxide with controlled species of oxygenated groups[J]. Chemical Science, 2016, 7（3）：1874-1881.

[45]　Dong L, Chen Z X, Lin S, et al. Reactivity-controlled preparation of ultralarge graphene oxide by chemical expansion of graphite[J]. Chemistry of Materials, 2017, 29（2）：564-572.

[46]　Dimiev A M, Tour J M. Mechanism of graphene oxide formation[J]. ACS Nano, 2014, 8（3）：3060-3068.

[47]　Sun H Y, Xu Z, Gao C. Multifunctional, ultra-flyweight, synergistically assembled carbon aerogels[J]. Advanced Materials, 2013, 25（18）：2554-2560.

[48]　Shin H J, Kim K K, Benayad A, et al. Efficient reduction of graphite oxide by sodium borohydride and its effect on electrical conductance[J]. Advanced Functional Materials, 2009, 19（12）：1987-1992.

[49]　Chua C K, Pumera M. Chemical reduction of graphene oxide：A synthetic chemistry viewpoint[J]. Chemical Society Reviews, 2014, 43（1）：291-312.

[50]　Xu Y X, Sheng K X, Li C, et al. Self-assembled graphene hydrogel via a one-step hydrothermal process[J]. ACS Nano, 2010, 4（7）：4324-4330.

[51]　Peng L, Xu Z, Liu Z, et al. Ultrahigh thermal conductive yet superflexible graphene films[J]. Advanced Materials, 2017, 29（27）：1700589.

[52]　Pei S F, Cheng H M. The reduction of graphene oxide[J]. Carbon, 2012, 50（9）：3210-3228.

[53]　Chen Y N, Fu K, Zhu S Z, et al. Reduced graphene oxide films with ultrahigh conductivity as Li-ion battery current collectors[J]. Nano Letters, 2016, 16（6）：3616-3623. jo4hzI/EJIiUVLxeV7NIMyF6zFxVvwwtUPuIRfWrnXlw9YBc3iMLdb9HsuvghSlH